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Room-Temperature, Highly Durable Ti3C2Tx MXene/Graphene Hybrid Fibers for NH3 Gas Sensing

Title
Room-Temperature, Highly Durable Ti3C2Tx MXene/Graphene Hybrid Fibers for NH3 Gas Sensing
Author
엄원식
Keywords
MXene; graphene oxide; wet-spinning; fiber assembly; NH3 gas sensors
Issue Date
2020-03
Publisher
AMER CHEMICAL SOC
Citation
ACS APPLIED MATERIALS & INTERFACES, v. 12, NO 9, Page. 10434-10442
Abstract
Graphene-based fibers (GFs) have aroused enormous interest in portable, wearable electronics because of their excellent mechanical flexibility, electrical conductivity, and weavability, which make them advantageous for wearable electronic devices. Herein, we report the development of metal binder-free Ti3C2Tx MXene/graphene hybrid fibers by a scalable wet-spinning process. These hybrid fibers exhibit excellent mechanical and electrical properties for applications in flexible wearable gas sensors. The synergistic effects of electronic properties and gas-adsorption capabilities of MXene/graphene allow the created fibers to show high NH3 gas sensitivity at room temperature. The hybrid fibers exhibited significantly improved NH3 sensing response (Delta R/R-0 = 6.77%) compared with individual MXene and graphene. The hybrid fibers also showed excellent mechanical flexibility with a minimal fluctuation of resistance of +/- 0.2% and low noise resistance even after bending over 2000 cycles, enabling gas sensing during deformation. Furthermore, flexible MXene/graphene hybrid fibers were woven into a lab coat, demonstrating their high potential for wearable devices. We envisage that these exciting features of 2D hybrid materials will provide a novel pathway for designing next-generation portable wearable gas sensors.
URI
https://pubs.acs.org/doi/10.1021/acsami.9b21765https://repository.hanyang.ac.kr/handle/20.500.11754/162800
ISSN
1944-8244; 1944-8252
DOI
10.1021/acsami.9b21765
Appears in Collections:
RESEARCH INSTITUTE[S](부설연구소) > RESEARCH INSTITUTE OF INDUSTRIAL SCIENCE(산업과학연구소) > Articles
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