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Long-term air-stable Au doping of graphene by layer-by-layer assembly with graphene oxide for flexible transparent electrodes

Title
Long-term air-stable Au doping of graphene by layer-by-layer assembly with graphene oxide for flexible transparent electrodes
Author
박진성
Keywords
Graphene; Graphene oxide; Doping; Flexible transparent electrodes
Issue Date
2018-01
Publisher
PERGAMON-ELSEVIER SCIENCE LTD
Citation
CARBON, v. 126, page. 241-246
Abstract
In order to realize the most suitable hybrid structure for air-stable graphene-based transparent and flexible electrodes, we systematically compared graphene oxide (GO)/Au/graphene and graphene/Au/GO hybrid films fabricated by layer-by-layer assembly. The sheet resistance of graphene/Au/GO was proportional to the concentration of AuCl3 (1-5 mg/ml), which can be understood by a significant blue-shift in the G-band associated with the phonon stiffening. The size and density of formed Au nanoparticles strongly influenced their reduction reaction, which is a crucial factor for maximizing the doping effects. The optimized optical transmittance and sheet resistance of GO/Au/graphene were 94.9% and 198 +/- 29 Ohm/sq, respectively. Furthermore, the hybrid films revealed stable doping effects (sheet resistance variation: 23-55%) against ambient conditions after 1 month. The variation in sheet resistance for GO/Au/graphene hybrid films corresponds to 30% with a bending radius of 10 mm after repeated bending tests (bending cycles of 10(5)). (C) 2017 Elsevier Ltd. All rights reserved.
URI
https://www.sciencedirect.com/science/article/pii/S0008622317309879?via%3Dihubhttp://repository.hanyang.ac.kr/handle/20.500.11754/117100
ISSN
0008-6223; 1873-3891
DOI
10.1016/j.carbon.2017.09.108
Appears in Collections:
COLLEGE OF ENGINEERING[S](공과대학) > MATERIALS SCIENCE AND ENGINEERING(신소재공학부) > Articles
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